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Preheat the oven to 350 degrees Fahrenheit. Grease two loaf pans with butter or nonstick cooking spray. Pay special attention to the corners of the pans to prevent sticking.
In a large mixing bowl, cream together the softened butter, 2 cups sugar, and eggs until light and fluffy. Stir in the vanilla extract.
Gradually add the buttermilk, flour, and baking soda to the wet mixture. Mix gently until everything is well combined.
In a separate bowl, combine ⅔ cup of sugar, ground cinnamon, and nutmeg. Mix well.
Divide the batter into four equal parts. Spread one-quarter of the batter into the bottom of each loaf pan. (Half of the batter in total for both pans.) Evenly sprinkle three-quarters of the cinnamon sugar mixture over the batter in each pan.
Spread the remaining batter over the cinnamon layer, dividing evenly between both pans.
Sprinkle the remaining cinnamon sugar mixture on top. Use a knife to gently swirl the batter and cinnamon sugar together to create a marbled effect.
Place the loaf pans in the preheated oven and bake for 45 to 50 minutes. Check for doneness by inserting a toothpick into the center of the bread. It should come out clean.
Allow the bread to cool in the pans for about 20 minutes. Then, remove the loaves from the pans and transfer them to a wire rack to cool completely. Enjoy!