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Heat oven to 200°F. Line large rimmed baking sheet with parchment paper.
Place popcorn in large bowl next to stove. In small saucepan, combine sugar, butter, corn syrup, molasses, and apple pie spice. While stirring, bring sugar mixture to a boil. Boil 5 minutes, stirring. Stir in baking soda, then immediately pour over popcorn. Using silicone spatula, fold caramel into popcorn to coat, then spread on prepared baking sheet. Sprinkle with salt.
Bake popcorn, stirring every 15 minutes, until caramel is dried and no longer sticky, about 1 hour. Transfer baking sheet to wire rack and let caramel corn cool to room temperature, then refrigerate until cold.